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When I redid some steel wheels I did the following:

1) remove wheel from car and mask off tire with newspaper and tape
2) sand entire wheel until it is smooth
3) clean wheel to remove all sanding dust
4) spray wheel with rustoleum white primer (2 coats)
5) spray wheel with light coats of rustoleum gloss black (as many coats as it takes to completely cover wheel)

They looked brand new. I then put on some stainless steel trim rings and bolted them to the car with chrome lug nuts.

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